Metamaterial plasmonic absorber for reducing the spectral shift between near- and far-field responses in surface-enhanced spectroscopy applications

Asian E., Aslan E., TÜRKMEN M., SARAÇOĞLU Ö. G.

SENSORS AND ACTUATORS A-PHYSICAL, vol.267, pp.60-69, 2017 (SCI-Expanded) identifier identifier

  • Publication Type: Article / Article
  • Volume: 267
  • Publication Date: 2017
  • Doi Number: 10.1016/j.sna.2017.10.006
  • Journal Indexes: Science Citation Index Expanded (SCI-EXPANDED), Scopus
  • Page Numbers: pp.60-69
  • Keywords: Nanophotonics, Metamaterials, Plasmonic absorbers, Molecular sensing, Surface enhanced infrared absorption spectroscopy (SEIRAS), INFRARED-ABSORPTION SPECTROSCOPY, PERFECT ABSORBER, ANTENNAS, NANOANTENNAS, ARRAYS, RESONANCES
  • Erciyes University Affiliated: Yes


The spectral shift between near- and far-field responses of the plasmonic nanoantennas has negative effects on the performance of surface-enhanced spectroscopy measurements. In order to reduce these effects, we propose use of the plasmonic absorber (PA) concept that promises lower spectral-shift between the near- and far-field responses. In this context, we present the design, characterization and experimental realization of a novel PA structure which utilizes hexagonally arranged nanoantennas operating in the mid-infrared regime. Additionally, we analyze the PA device numerically and experimentally to investigate tunability of resonant modes. To reveal the absorption mechanism, we investigate the near-field distribution maps in addition to the charge and current density distributions. With the aim of comparing the proposed PA device with the conventional particle-based nanoantenna according to the amount of spectral shift between the near- and far-field peaks, we present the near- and far-field spectra of each configuration and show that PA structure exhibits significantly lower spectral-shift. Finally, we present the effect of reduced spectral-shift on the surface-enhanced infrared absorption spectroscopy through the simulations for the detection of the molecular absorption mode of a polymer and compare with the results of particle nanoantenna configuration. (C) 2017 Elsevier B.V. All rights reserved.